Arno Anzenbacher Pdf Viewer

Synopsis A series of blue-emitting 5-substituted bis(2-methyl-8-quinolinolate)phenolate aluminum(III) complexes were synthesized, and their electrochemical and optical properties were investigated. When electron-withdrawing moieties are attached to the 5-position of the ligand, a blue emission (460−480 nm) is obtained. The effect of the substituents on the emission can be predicted with a high degree of accuracy using a density functional theory method (DFT/B3LYP/6-31G*). These complexes may be suitable as materials for organic light-emitting (OLED) device fabrication. Blue-emitting heteroleptic aluminum(III) bis(2-methyl-8-quinolinolate)phenolate complexes were synthesized. A tunable, blue-to-green emission is achieved by attaching electron-withdrawing modulators to the emisssive quinaldinate ligand.

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The electronic nature of modulator substituents attached to the position of the highest HOMO (highest occupied molecular orbital) density is used to modulate ligand HOMO levels to achieve effective emission tuning to obtain blue-emitting materials. Optical and electrochemical properties of the resulting complexes were investigated and compared to the results of density functional theory (DFT/B3LYP/6-31G*) studies. The resulting materials may find application as organic light-emitting device materials.

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